@article{10902/28109,
year = {2022},
month = {10},
url = {https://hdl.handle.net/10902/28109},
abstract = {We study the emergence of Berezinskii-Kosterlitz-Thouless (BKT) phases in (PbTiO3 )3/(SrTiO3 )3 superlattices by means of second-principles simulations. Between a tensile epitaxial strain of _ = 0.25?1%, the local dipole moments within the superlattices are confined to the film-plane, and thus the polarization can be effectively considered as two-dimensional. The analysis of the decay of the dipole-dipole correlation with the distance, together with the study of the density of defects and its distribution as a function of temperature, supports the existence of a BKT phase in a range of temperature mediating the ordered ferroelectric (stable at low T ), and the disordered paraelectric phase that appears beyond a critical temperature TBKT. This BKT phase is characterized by quasi-long-range order (whose signature is a power-law decay of the correlations with the distance), and the emergence of tightly bound vortex-antivortex pairs whose density is determined by a thermal activation process. The proposed PbTiO3/SrTiO3 superlattice model and the imposed mechanical boundary conditions are both experimentally feasible, making it susceptible for an experimental observation of these new topological phases in ferroelectric materials.},
organization = {F.G.-O., P.G.-F., and J.J. acknowledge financial support from Grant No. PGC2018-096955-B-C41 funded by MCIN/AEI/10.13039/501100011033 and by ERDF “A way of making Europe” by the European Union. F.G.-O. acknowledges financial support from Grant No. FPU18/04661 funded by MCIN/AEI/10.13039/501100011033.},
publisher = {American Physical Society},
publisher = {Physical Review B, 2022, 106(13), 134106},
title = {Berezinskii-Kosterlitz-Thouless phases in ultrathin PbTiO3/SrTiO3 superlattices},
author = {Gómez Ortiz, Fernando and García Fernández, Pablo (físico) and López Martín, Juan Manuel and Junquera Quintana, Francisco Javier},
}